When Do You Stop Link Building

Only as long as your site is crap and can't attract natural backlinks I guess? ;)

If you can get natural backlinks automatically, then you don't need to fake any backlinks. This only happens to those with good sites, that have ever green content though. What is your site based on?
Totally agree. Also curious about OP's website!
 
Eventually, there comes a time when building extra backlinks doesn’t make any difference to your page. Is there a limit to how many links you can build, beyond which you start working on content optimization?
There is no link count where it stops, so stop looking for a number. Watch the response instead. Log the position before and after each batch, and if two batches of similar quality move nothing, links are not what is holding the page back. Then it is usually an intent mismatch, the wrong page type for that SERP, or content missing the subtopics the ranking pages cover.

Also don't drop links to zero. Links churn and competitors keep adding, so on a contested term a page that stops completely tends to slide slowly. Go to a maintenance trickle and put the main effort into the page.
 
Cease link-building activities when: your backlink profile shows signs of irregularities or has been subject to penalties; content quality and on-page SEO standards fall short of requirements; link metrics have reached a point of industry saturation; or the website shifts toward a strategy focused on "earning" links naturally.
 
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